A new approach to ferrocene derived alkenes via coppercatalyzed olefination

A new approach to ferrocenyl haloalkenes and bis-alkenes was elaborated. The key procedure involves copper catalyzed olefination of N-unsubstituted hydrazones, obtained from ferrocene-containing carbonyl compounds and hydrazine, with polyhaloalkanes. The procedure is simple, cheap and could be applied for the utilization of environmentally harmful polyhalocarbons. The cyclic voltammetry study of the representative examples of the synthesized ferrocenyl alkenes shows the strong dependence of the cathodic behavior on the amount of vinyl groups: while for the monoalkene containing molecules no reduction is seen, the divinyl products are reduced in several steps. © 2015 Muzalevskiy et al; licensee Beilstein-Institut.

Авторы
Muzalevskiy V.M.1 , Shastin A.V.1, 2 , Demidovich A.D.1 , Shikhaliev N.G.3 , Magerramov A.M.3 , Khrustalev V.N. 4, 5 , Rakhimov R.D.1 , Vatsadze S.Z.1 , Nenajdenko V.G.1, 5
Издательство
Beilstein-Institut Zur Forderung der Chemischen Wissenschaften
Язык
Английский
Страницы
2072-2078
Статус
Опубликовано
Том
11
Год
2015
Организации
  • 1 Department of Chemistry, Lomonosov Moscow State University, Moscow, 119991, Russian Federation
  • 2 Institute of Problems of Chemical Physics, Russian Academy of Sciences, Chernogolovka, Moscow Region, 142432, Russian Federation
  • 3 Baku State University, Department of Chemistry, Z. Xalilov Str. 23, Baku, Az 1148, Azerbaijan
  • 4 Peoples' Friendship University of Russia, 28 Vavilov Street, Moscow, 119991, Russian Federation
  • 5 A.N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, 28 Vavilov Street, Moscow, 119991, Russian Federation
Ключевые слова
Catalytic olefination; Copper catalysis; Cyclic voltammetry; Ferrocene
Дата создания
19.10.2018
Дата изменения
19.10.2018
Постоянная ссылка
https://repository.rudn.ru/ru/records/article/record/4487/
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